Publicação
Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds
| Resumo: | Environmentally resilient antimicrobial coatings are becoming increasingly required for a wide range of applications. For this purpose, nanocomposite thin films of poly(vinylidene fluoride) (PVDF) filled with several types of functionalized nanodiamonds (NDs) were processed by solvent casting. The effects of ND inclusion and functionalization in their morphological, structural, optical, thermal, and electrical properties were evaluated taking into account the type of the nanofiller and a concentration up to 2 wt %. The morphology, structure, and thermal features of the polymer matrix are governed by the processing conditions, and no noticeable changes occurred due to the presence of the ND fillers. The polymer crystallized mainly in the α phase with a crystallinity of ≈60%. In turn, the optical transmittance from 200 to 800 nm and the dielectric constant effectively depended on the ND type and content. The inclusion of the ND particles effectively provided antimicrobial properties to the films, which depended on the ND functionalization. This study thus shows that the incorporation of functionalized NDs into PVDF allows the development of antimicrobial coatings with tailorable optical and dielectric properties, which could be of great importance to face nowadays pandemic crisis scenario. |
|---|---|
| Autores principais: | Nunes-Pereira, João |
| Outros Autores: | Costa, Pedro; Fernandes, Liliana; Carvalho, Estela O.; Fernandes, Margarida M.; Carabineiro, S.A.C.; Buijnsters, Josephus; Rial Tubio, Carmen; Lanceros-Mendez, Senentxu |
| Assunto: | Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| Ano: | 2020 |
| País: | Portugal |
| Tipo de documento: | artigo |
| Tipo de acesso: | acesso restrito |
| Instituição associada: | Universidade da Beira Interior |
| Idioma: | inglês |
| Origem: | uBibliorum |
| _version_ | 1868420947783974912 |
|---|---|
| author | Nunes-Pereira, João |
| author2 | Costa, Pedro Fernandes, Liliana Carvalho, Estela O. Fernandes, Margarida M. Carabineiro, S.A.C. Buijnsters, Josephus Rial Tubio, Carmen Lanceros-Mendez, Senentxu |
| author2_role | author author author author author author author author |
| author_facet | Nunes-Pereira, João Costa, Pedro Fernandes, Liliana Carvalho, Estela O. Fernandes, Margarida M. Carabineiro, S.A.C. Buijnsters, Josephus Rial Tubio, Carmen Lanceros-Mendez, Senentxu |
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| datacite.creators.creator.creatorName.fl_str_mv | Nunes-Pereira, João Costa, Pedro Fernandes, Liliana Carvalho, Estela O. Fernandes, Margarida M. Carabineiro, S.A.C. Buijnsters, Josephus Rial Tubio, Carmen Lanceros-Mendez, Senentxu |
| datacite.date.Accepted.fl_str_mv | 2020-01-01T00:00:00Z |
| datacite.date.available.fl_str_mv | 2024-02-26T11:15:27Z |
| datacite.date.embargoed.fl_str_mv | 2024-02-26T11:15:27Z |
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| datacite.subjects.subject.fl_str_mv | Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| datacite.titles.title.fl_str_mv | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| dc.contributor.none.fl_str_mv | uBibliorum |
| dc.creator.none.fl_str_mv | Nunes-Pereira, João Costa, Pedro Fernandes, Liliana Carvalho, Estela O. Fernandes, Margarida M. Carabineiro, S.A.C. Buijnsters, Josephus Rial Tubio, Carmen Lanceros-Mendez, Senentxu |
| dc.date.Accepted.fl_str_mv | 2020-01-01T00:00:00Z |
| dc.date.available.fl_str_mv | 2024-02-26T11:15:27Z |
| dc.date.embargoed.fl_str_mv | 2024-02-26T11:15:27Z |
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| dc.language.none.fl_str_mv | eng |
| dc.publisher.none.fl_str_mv | https://pubs.acs.org/doi/10.1021/acsapm.0c00869?ref=pdf |
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| dc.rights.none.fl_str_mv | http://purl.org/coar/access_right/c_16ec |
| dc.subject.none.fl_str_mv | Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| dc.title.fl_str_mv | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| dc.type.none.fl_str_mv | http://purl.org/coar/resource_type/c_6501 |
| description | Environmentally resilient antimicrobial coatings are becoming increasingly required for a wide range of applications. For this purpose, nanocomposite thin films of poly(vinylidene fluoride) (PVDF) filled with several types of functionalized nanodiamonds (NDs) were processed by solvent casting. The effects of ND inclusion and functionalization in their morphological, structural, optical, thermal, and electrical properties were evaluated taking into account the type of the nanofiller and a concentration up to 2 wt %. The morphology, structure, and thermal features of the polymer matrix are governed by the processing conditions, and no noticeable changes occurred due to the presence of the ND fillers. The polymer crystallized mainly in the α phase with a crystallinity of ≈60%. In turn, the optical transmittance from 200 to 800 nm and the dielectric constant effectively depended on the ND type and content. The inclusion of the ND particles effectively provided antimicrobial properties to the films, which depended on the ND functionalization. This study thus shows that the incorporation of functionalized NDs into PVDF allows the development of antimicrobial coatings with tailorable optical and dielectric properties, which could be of great importance to face nowadays pandemic crisis scenario. |
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| person_str_mv | Nunes-Pereira, João Nunes-Pereira, João https://www.ciencia-id.pt/6D16-6F7E-64F0 6D16-6F7E-64F0 http://orcid.org/0000-0002-6024-8716 0000-0002-6024-8716 Costa, Pedro Costa, Pedro https://www.ciencia-id.pt/7E1E-A2E1-0E73 7E1E-A2E1-0E73 http://orcid.org/0000-0001-9887-0925 0000-0001-9887-0925 Fernandes, Liliana Fernandes, Liliana https://www.ciencia-id.pt/2B1B-04B1-6F9E 2B1B-04B1-6F9E http://orcid.org/0000-0002-5428-4411 0000-0002-5428-4411 Carvalho, Estela O. Carvalho, Estela O. https://www.ciencia-id.pt/331D-16E7-FF9C 331D-16E7-FF9C http://orcid.org/0000-0002-6110-9814 0000-0002-6110-9814 Fernandes, Margarida M. Fernandes, Margarida M. https://www.ciencia-id.pt/3B1C-A9A1-EC3E 3B1C-A9A1-EC3E http://orcid.org/0000-0002-1529-3702 0000-0002-1529-3702 Carabineiro, S.A.C. Carabineiro, S.A.C. https://www.ciencia-id.pt/1212-CC72-1B41 1212-CC72-1B41 http://orcid.org/0000-0001-9913-4671 0000-0001-9913-4671 Buijnsters, Josephus Buijnsters, Josephus http://orcid.org/0000-0002-5440-8154 0000-0002-5440-8154 Rial Tubio, Carmen Rial Tubio, Carmen https://www.ciencia-id.pt/0612-C48A-92D9 0612-C48A-92D9 http://orcid.org/0000-0002-6988-8242 0000-0002-6988-8242 Lanceros-Mendez, Senentxu Lanceros-Mendez, Senentxu https://www.ciencia-id.pt/8318-953C-0D4D 8318-953C-0D4D http://orcid.org/0000-0001-6791-7620 0000-0001-6791-7620 |
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| spelling | enghttps://pubs.acs.org/doi/10.1021/acsapm.0c00869?ref=pdfpt_PTEnvironmentally resilient antimicrobial coatings are becoming increasingly required for a wide range of applications. For this purpose, nanocomposite thin films of poly(vinylidene fluoride) (PVDF) filled with several types of functionalized nanodiamonds (NDs) were processed by solvent casting. The effects of ND inclusion and functionalization in their morphological, structural, optical, thermal, and electrical properties were evaluated taking into account the type of the nanofiller and a concentration up to 2 wt %. The morphology, structure, and thermal features of the polymer matrix are governed by the processing conditions, and no noticeable changes occurred due to the presence of the ND fillers. The polymer crystallized mainly in the α phase with a crystallinity of ≈60%. In turn, the optical transmittance from 200 to 800 nm and the dielectric constant effectively depended on the ND type and content. The inclusion of the ND particles effectively provided antimicrobial properties to the films, which depended on the ND functionalization. This study thus shows that the incorporation of functionalized NDs into PVDF allows the development of antimicrobial coatings with tailorable optical and dielectric properties, which could be of great importance to face nowadays pandemic crisis scenario.application/pdfpt_PTAntimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized NanodiamondsPersonalNunes-Pereira, JoãoDSpacehttp://dspace.org/items/6c577fb3-3c47-4e95-87f0-85484f1734ffDSpacehttp://dspace.org/items/6c577fb3-3c47-4e95-87f0-85484f1734ffNunes-PereiraJoãoCiência IDhttps://www.ciencia-id.pt6D16-6F7E-64F0ORCIDhttp://orcid.org0000-0002-6024-8716Researcher IDhttps://www.researcherid.comAAD-6349-2020Scopus Author IDhttps://www.scopus.com57200519831PersonalCosta, PedroDSpacehttp://dspace.org/items/1d582288-b555-4cc1-b912-76c44e9a1c55DSpacehttp://dspace.org/items/1d582288-b555-4cc1-b912-76c44e9a1c55CostaPedroCiência IDhttps://www.ciencia-id.pt7E1E-A2E1-0E73ORCIDhttp://orcid.org0000-0001-9887-0925Scopus Author IDhttps://www.scopus.com56335530700PersonalFernandes, LilianaDSpacehttp://dspace.org/items/205c6ccc-4b77-4ae8-aceb-e7c79d7ba788DSpacehttp://dspace.org/items/205c6ccc-4b77-4ae8-aceb-e7c79d7ba788FernandesLilianaCiência IDhttps://www.ciencia-id.pt2B1B-04B1-6F9EORCIDhttp://orcid.org0000-0002-5428-4411Scopus Author IDhttps://www.scopus.com56045917800PersonalCarvalho, Estela O.DSpacehttp://dspace.org/items/f0e16307-447b-4936-bf36-a492f13f3010DSpacehttp://dspace.org/items/f0e16307-447b-4936-bf36-a492f13f3010CarvalhoEstela O.Ciência IDhttps://www.ciencia-id.pt331D-16E7-FF9CORCIDhttp://orcid.org0000-0002-6110-9814Scopus Author IDhttps://www.scopus.com57197713772PersonalFernandes, Margarida M.DSpacehttp://dspace.org/items/ba166b1d-465a-4a95-ae41-41ea6d87716aDSpacehttp://dspace.org/items/ba166b1d-465a-4a95-ae41-41ea6d87716aFernandesMargaridaCiência IDhttps://www.ciencia-id.pt3B1C-A9A1-EC3EORCIDhttp://orcid.org0000-0002-1529-3702Researcher IDhttps://www.researcherid.comT-8132-2018Scopus Author IDhttps://www.scopus.com57207806661PersonalCarabineiro, S.A.C.DSpacehttp://dspace.org/items/e237c4d2-db8d-4acd-97da-9e1dbc6bc84eDSpacehttp://dspace.org/items/e237c4d2-db8d-4acd-97da-9e1dbc6bc84eCorreia CarabineiroSónia AlexandraCiência IDhttps://www.ciencia-id.pt1212-CC72-1B41ORCIDhttp://orcid.org0000-0001-9913-4671Scopus Author IDhttps://www.scopus.com6602118574PersonalBuijnsters, JosephusDSpacehttp://dspace.org/items/71fba4b1-af14-49c4-b88a-39a9ae3d5f8cDSpacehttp://dspace.org/items/71fba4b1-af14-49c4-b88a-39a9ae3d5f8cBuijnstersJosephusORCIDhttp://orcid.org0000-0002-5440-8154Scopus Author IDhttps://www.scopus.com6602876650PersonalRial Tubio, CarmenDSpacehttp://dspace.org/items/608b43eb-099d-47e3-a39a-a97b3ff7cad6DSpacehttp://dspace.org/items/608b43eb-099d-47e3-a39a-a97b3ff7cad6Rial TubioCarmenCiência IDhttps://www.ciencia-id.pt0612-C48A-92D9ORCIDhttp://orcid.org0000-0002-6988-8242Researcher IDhttps://www.researcherid.comM-5829-2018Scopus Author IDhttps://www.scopus.com26032414000PersonalLanceros-Mendez, SenentxuDSpacehttp://dspace.org/items/29aa0540-09be-4772-a9af-d03e10a6b574DSpacehttp://dspace.org/items/29aa0540-09be-4772-a9af-d03e10a6b574Lanceros-MendezSenentxuCiência IDhttps://www.ciencia-id.pt8318-953C-0D4DORCIDhttp://orcid.org0000-0001-6791-7620HostingInstitutionOrganizationaluBibliorume-mailmailto:noreplyuBibliorum@ubi.ptnoreplyuBibliorum@ubi.ptDOIIsPartOf10.1021/acsapm.0c008692024-02-26T11:15:27Z20202020-01-01T00:00:00ZHandlehttp://hdl.handle.net/10400.6/14261http://purl.org/coar/access_right/c_16ecrestricted accessNanodiamondsPoly (vinylidene fluoride)Solvent castingAntimicrobial filmsPolymer composites6244610 bytesFundação para a Ciência e a TecnologiaC-MAST - 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| spellingShingle | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds Nunes-Pereira, João Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| status | SINGLETON |
| subject.fl_str_mv | Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| title | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| title_full | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| title_fullStr | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| title_full_unstemmed | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| title_short | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| title_sort | Antimicrobial and Antibiofilm Properties of Fluorinated Polymers with Embedded Functionalized Nanodiamonds |
| topic | Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| topic_facet | Nanodiamonds Poly (vinylidene fluoride) Solvent casting Antimicrobial films Polymer composites |
| url | http://hdl.handle.net/10400.6/14261 |
| visible | 1 |